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Fabrication of Eco-Friendly Solid-State Symmetric Ultracapacitor Device Based on Co-Doped PANI/GO Composite

Affiliation
Conductive Polymers and Electrochemistry Laboratory, National Centre of Excellence in Physical Chemistry, University of Peshawar, Peshawar 25120, Pakistan.
Gul, Hajera;
GND
133118258
Affiliation
Physical Chemistry Laboratory, Institute of Chemical Sciences, University of Peshawar, Peshawar 25120, Pakistan. s.bilal@tu-braunschweig.de.
Shah, Anwar-ul-Haq Ali;
GND
133643379
Affiliation
Conductive Polymers and Electrochemistry Laboratory, National Centre of Excellence in Physical Chemistry, University of Peshawar, Peshawar 25120, Pakistan. salmabilal@uop.edu.pk.
Bilal, Salma

An eco-friendly solid-state symmetric ultracapacitor (Uc) device was fabricated using a polyaniline graphene oxide composite co-doped with sulfuric acid (H2SO4) and dodecyl benzene sulfonic acid (DBSA) or camphor sulfonic acid (CSA), as electrode material utilizing gold sheets as current collectors. The device showed specific capacitance value of 150 F/g at 1 A/g current density, with a capacitance retention value of 93.33% at higher current density (10 A/g), indicating a high rate capability. An energy density of 15.30 Whkg-1 with a power density of 1716 Wkg-1 was obtained at the current density of 1 A/g. The values of areal capacitance, power density, and energy density, achieved at the current density of 5 mAcm-2, were 97.38 mFcm-2, 9.93 mWhcm-2, and 1.1 Wcm-2, respectively. Additionally, the device showed very low solution and charge transfer resistance (0.885 Ω and 0.475 Ω, respectively). A device was also fabricated utilizing copper as current collector; however, a lower value of specific capacitance (82 F/g) was observed in this case.

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